Fibre-metal laminates (FMLs) represent high-performance hybrid composites that couple the impact toughness and ductility of metals with the high stiffness and specific strength of fibre-reinforced polymers. Although aluminium-based FMLs like ARALL and GLARE have seen extensive use, their galvanic corrosion, heat management, and crack growth limitations limit their long-term reliability. Titanium-based FMLs (Ti-FMLs) overcome these challenges with enhanced corrosion resistance, toughness, and high-performance fibre compatibility, positioning them as prime contenders for aerospace, automotive, and marine applications where weight optimization and durability are paramount. Yet, experimental testing of Ti-FMLs is still expensive and time-consuming, pointing to a requirement for computational methods to estimate their structural response under various conditions. This paper applies finite element analysis (FEA) with the ANSYS package, supported by CADEC material modelling, to model the interaction between titanium layers and Zylon–epoxy composites. The methodology is aimed at confirming experimental results, evaluating behaviour under static and changing loading conditions, and enhancing knowledge of stress distribution, deformation, and failure mechanisms.Through rigorous combination with experimental verification, this research pushes the predictive design of Ti-FMLs to their mechanical behaviour and optimisation for ultra-high-performance engineering systems. The findings are anticipated to advance the establishment of light, resilient materials that can fulfil the high requirements of next-generation aerospace and marine applications.